TY - JOUR
T1 - Stochastic Phase Transition Dynamics in Nonequilibrium System
T2 - Holographic Study
AU - Pagnacco, Maja C.
AU - Simović-Pavlović, Marina
AU - Grujić, Dušan Ž
AU - Vasiljević, Darko M.
AU - Bokic, Bojana
AU - Mouchet, Sébastien R.
AU - Verbiest, Thierry
AU - Caudano, Yves
AU - Kolaric, Branko
N1 - Funding Information:
M.S.P., D.Ž.G., D.V., and B.K. acknowledge support of the project Biological and bioinspired structures for multispectral surveillance, funded by NATO SPS (NATO Science for Peace and Security) 2019-2022. B.K., D.V., B.B., D.Ž.G., and M.S.-P. acknowledge funding provided by the Institute of Physics Belgrade, through the institutional funding by the Ministry of Education, Science, and Technological Development of the Republic of Serbia. Y.C. is a research associate of the Fund for Scientific Research F.R.S.-FNRS. Additionally, B.K. acknowledges support from F.R.S.-FNRS. M.C.P. acknowledges support from the Ministry of Education, Science and Technological Development of the Republic of Serbia, Contract number 451-03-9/2021-14/200026. S.R.M. was supported by a BEWARE Fellowship (Convention no. 2110034) of the Walloon Region (Marie Skłodowska-Curie Actions of the European Union - COFUND - contract 847587), as a postdoctoral researcher. T.V. acknowledges financial support from the Hercules Foundation. D.V., M.S.P., D.Ž.G., M.P., B.B., and B.K. acknowledge the support of the Office of Naval Research Global through the Research Grant N62902-22-1-2024.
Funding Information:
M.S.P., D.Ž.G., D.V., and B.K. acknowledge support of the project Biological and bioinspired structures for multispectral surveillance, funded by NATO SPS (NATO Science for Peace and Security) 2019–2022. B.K., D.V., B.B., D.Ž.G., and M.S.-P. acknowledge funding provided by the Institute of Physics Belgrade, through the institutional funding by the Ministry of Education, Science, and Technological Development of the Republic of Serbia. Y.C. is a research associate of the Fund for Scientific Research F.R.S.-FNRS. Additionally, B.K. acknowledges support from F.R.S.-FNRS. M.C.P. acknowledges support from the Ministry of Education, Science and Technological Development of the Republic of Serbia, Contract number 451-03-9/2021-14/200026. S.R.M. was supported by a BEWARE Fellowship (Convention no. 2110034) of the Walloon Region (Marie Skłodowska-Curie Actions of the European Union - COFUND - contract 847587), as a postdoctoral researcher. T.V. acknowledges financial support from the Hercules Foundation. D.V., M.S.P., D.Ž.G., M.P., B.B., and B.K. acknowledge the support of the Office of Naval Research Global through the Research Grant N62902-22-1-2024.
Publisher Copyright:
© 2023 American Chemical Society.
PY - 2023/6/8
Y1 - 2023/6/8
N2 - This paper presents a holographic study of the phase transition that occurs in a nonequilibrium system. The chosen model is a unique Briggs-Rauscher oscillatory reaction that, first, follows a deterministic pattern (namely, an oscillatory behavior) and, later, exhibits a phase transition occurring randomly and without any known link with the previous deterministic state. The presented research opens up a new way to reveal complex chemical phenomena and dynamics in situ, without disturbing significantly the nonequilibrium system and its pathways. Simultaneously, it unfolds a new route for applications of interferometric methods in different areas of materials science. Under the applied conditions, we show that the holographic method is more sensitive to the phase transition dynamics than the commonly used potentiometric method.
AB - This paper presents a holographic study of the phase transition that occurs in a nonequilibrium system. The chosen model is a unique Briggs-Rauscher oscillatory reaction that, first, follows a deterministic pattern (namely, an oscillatory behavior) and, later, exhibits a phase transition occurring randomly and without any known link with the previous deterministic state. The presented research opens up a new way to reveal complex chemical phenomena and dynamics in situ, without disturbing significantly the nonequilibrium system and its pathways. Simultaneously, it unfolds a new route for applications of interferometric methods in different areas of materials science. Under the applied conditions, we show that the holographic method is more sensitive to the phase transition dynamics than the commonly used potentiometric method.
UR - http://www.scopus.com/inward/record.url?scp=85162747357&partnerID=8YFLogxK
U2 - 10.1021/acs.jpcc.3c01831
DO - 10.1021/acs.jpcc.3c01831
M3 - Article
AN - SCOPUS:85162747357
SN - 1932-7447
VL - 127
SP - 10821
EP - 10825
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 22
ER -