One-pot fabrication of FePt/reduced graphene oxide composites as highly active and stable electrocatalysts for the oxygen reduction reaction

Dan Chen, Xin Zhao, Shanshan Chen, Huifeng Li, Xinning Fu, Qingzhi Wu, Shipu Li, Yu Li, Bao Lian Su, Rodney S. Ruoff

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Résumé

FePt nanoparticles (NPs)/reduced graphene oxide (rG-O) composites have been synthesized using a one-pot strategy without surfactants. Monodisperse FePt NPs were homogenously loaded onto rG-O sheets. By controlling the concentration of dispersed graphene oxide (GO), uniform FePt flower-like nanoclusters can be obtained. FePt/rG-O composites exhibited exceptionally high electrocatalytic performance in the activity and durability for the oxygen reduction reaction (ORR), much superior to that of the commercial Pt/C (60%). The straightforward synthesis of FePt/rG-O composites provides a low-cost and high performance catalyst for the ORR, which is also a promising strategy for the synthesis of various Pt-based bimetallic alloy/rG-O composites for potential uses in catalysis and energy fields.

langue originaleAnglais
Pages (de - à)755-762
Nombre de pages8
journalCarbon
Volume68
Les DOIs
Etat de la publicationPublié - 1 mars 2014

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