Hierarchical MoS2@TiO2 Heterojunctions for Enhanced Photocatalytic Performance and Electrocatalytic Hydrogen Evolution

Yu Dong, Sheng You Chen, Yi Lu, Yu Xuan Xiao, Jie Hu, Si Ming Wu, Zhao Deng, Ge Tian, Gang Gang Chang, Jing Li, Silvia Lenaerts, Christoph Janiak, Xiao Yu Yang, Bao Lian Su

Résultats de recherche: Contribution à un journal/une revueArticle

Résumé

Hierarchical MoS2@TiO2 heterojunctions were synthesized through a one-step hydrothermal method by using protonic titanate nanosheets as the precursor. The TiO2 nanosheets prevent the aggregation of MoS2 and promote the carrier transfer efficiency, and thus enhance the photocatalytic and electrocatalytic activity of the nanostructured MoS2. The obtained MoS2@TiO2 has significantly enhanced photocatalytic activity in the degradation of rhodamine B (over 5.2 times compared with pure MoS2) and acetone (over 2.8 times compared with pure MoS2). MoS2@TiO2 is also beneficial for electrocatalytic hydrogen evolution (26 times compared with pure MoS2, based on the cathodic current density). This work offers a promising way to prevent the self-aggregation of MoS2 and provides a new insight for the design of heterojunctions for materials with lattice mismatches.

langue originaleAnglais
Pages (de - à)1609-1615
Nombre de pages7
journalChemistry - An Asian Journal
Volume13
Numéro de publication12
Les DOIs
étatPublié - 18 juin 2018

Empreinte digitale

rhodamine B
Nanosheets
Acetone
Heterojunctions
Hydrogen
Agglomeration
Lattice mismatch
Current density
Degradation

mots-clés

    Citer ceci

    Dong, Yu ; Chen, Sheng You ; Lu, Yi ; Xiao, Yu Xuan ; Hu, Jie ; Wu, Si Ming ; Deng, Zhao ; Tian, Ge ; Chang, Gang Gang ; Li, Jing ; Lenaerts, Silvia ; Janiak, Christoph ; Yang, Xiao Yu ; Su, Bao Lian. / Hierarchical MoS2@TiO2 Heterojunctions for Enhanced Photocatalytic Performance and Electrocatalytic Hydrogen Evolution. Dans: Chemistry - An Asian Journal. 2018 ; Vol 13, Numéro 12. p. 1609-1615.
    @article{bc6d3a477c7d45838af6133296211fd7,
    title = "Hierarchical MoS2@TiO2 Heterojunctions for Enhanced Photocatalytic Performance and Electrocatalytic Hydrogen Evolution",
    abstract = "Hierarchical MoS2@TiO2 heterojunctions were synthesized through a one-step hydrothermal method by using protonic titanate nanosheets as the precursor. The TiO2 nanosheets prevent the aggregation of MoS2 and promote the carrier transfer efficiency, and thus enhance the photocatalytic and electrocatalytic activity of the nanostructured MoS2. The obtained MoS2@TiO2 has significantly enhanced photocatalytic activity in the degradation of rhodamine B (over 5.2 times compared with pure MoS2) and acetone (over 2.8 times compared with pure MoS2). MoS2@TiO2 is also beneficial for electrocatalytic hydrogen evolution (26 times compared with pure MoS2, based on the cathodic current density). This work offers a promising way to prevent the self-aggregation of MoS2 and provides a new insight for the design of heterojunctions for materials with lattice mismatches.",
    keywords = "electrochemistry, hybrid structures, hydrogen, nanostructures, photochemistry, electron transfer, photocatalysts, naocomposites",
    author = "Yu Dong and Chen, {Sheng You} and Yi Lu and Xiao, {Yu Xuan} and Jie Hu and Wu, {Si Ming} and Zhao Deng and Ge Tian and Chang, {Gang Gang} and Jing Li and Silvia Lenaerts and Christoph Janiak and Yang, {Xiao Yu} and Su, {Bao Lian}",
    year = "2018",
    month = "6",
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    doi = "10.1002/asia.201800359",
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    Hierarchical MoS2@TiO2 Heterojunctions for Enhanced Photocatalytic Performance and Electrocatalytic Hydrogen Evolution. / Dong, Yu; Chen, Sheng You; Lu, Yi; Xiao, Yu Xuan; Hu, Jie; Wu, Si Ming; Deng, Zhao; Tian, Ge; Chang, Gang Gang; Li, Jing; Lenaerts, Silvia; Janiak, Christoph; Yang, Xiao Yu; Su, Bao Lian.

    Dans: Chemistry - An Asian Journal, Vol 13, Numéro 12, 18.06.2018, p. 1609-1615.

    Résultats de recherche: Contribution à un journal/une revueArticle

    TY - JOUR

    T1 - Hierarchical MoS2@TiO2 Heterojunctions for Enhanced Photocatalytic Performance and Electrocatalytic Hydrogen Evolution

    AU - Dong, Yu

    AU - Chen, Sheng You

    AU - Lu, Yi

    AU - Xiao, Yu Xuan

    AU - Hu, Jie

    AU - Wu, Si Ming

    AU - Deng, Zhao

    AU - Tian, Ge

    AU - Chang, Gang Gang

    AU - Li, Jing

    AU - Lenaerts, Silvia

    AU - Janiak, Christoph

    AU - Yang, Xiao Yu

    AU - Su, Bao Lian

    PY - 2018/6/18

    Y1 - 2018/6/18

    N2 - Hierarchical MoS2@TiO2 heterojunctions were synthesized through a one-step hydrothermal method by using protonic titanate nanosheets as the precursor. The TiO2 nanosheets prevent the aggregation of MoS2 and promote the carrier transfer efficiency, and thus enhance the photocatalytic and electrocatalytic activity of the nanostructured MoS2. The obtained MoS2@TiO2 has significantly enhanced photocatalytic activity in the degradation of rhodamine B (over 5.2 times compared with pure MoS2) and acetone (over 2.8 times compared with pure MoS2). MoS2@TiO2 is also beneficial for electrocatalytic hydrogen evolution (26 times compared with pure MoS2, based on the cathodic current density). This work offers a promising way to prevent the self-aggregation of MoS2 and provides a new insight for the design of heterojunctions for materials with lattice mismatches.

    AB - Hierarchical MoS2@TiO2 heterojunctions were synthesized through a one-step hydrothermal method by using protonic titanate nanosheets as the precursor. The TiO2 nanosheets prevent the aggregation of MoS2 and promote the carrier transfer efficiency, and thus enhance the photocatalytic and electrocatalytic activity of the nanostructured MoS2. The obtained MoS2@TiO2 has significantly enhanced photocatalytic activity in the degradation of rhodamine B (over 5.2 times compared with pure MoS2) and acetone (over 2.8 times compared with pure MoS2). MoS2@TiO2 is also beneficial for electrocatalytic hydrogen evolution (26 times compared with pure MoS2, based on the cathodic current density). This work offers a promising way to prevent the self-aggregation of MoS2 and provides a new insight for the design of heterojunctions for materials with lattice mismatches.

    KW - electrochemistry

    KW - hybrid structures

    KW - hydrogen

    KW - nanostructures

    KW - photochemistry

    KW - electron transfer

    KW - photocatalysts

    KW - naocomposites

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