Application of Green's Function theory to the calculation of ionization potentials of model oligomeric systems

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Résumé

The vertical ionization potentials of model hydrogen chains have been calculated, in the framework of STO-3G and 4-31G bases, at the second-order level of the many-body Green's function theory. Compared to the second-order many-body perturbation theory, this approach provides a qualitative description of trends observed with orbital relaxation, pair removal, and pair relaxation effects when studying oligomeric systems of increasing size with varying bond length.
langue originaleAnglais
Pages (de - à)243-255
Nombre de pages13
journalInternational Journal of Quantum Chemistry
Volume41
Numéro de publication2
Les DOIs
Etat de la publicationPublié - 1992

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