Quantum cascade laser dual-comb spectroscopy (DCS) for methane gas mixture studies

Muriel Lepère; Olivier Browet; Sylvain Leonis; Jean Clément; Pitt Allmendinger; Kuno Knapp; Florian Eigenmann; Markus Mangold

doi:10.1117/12.2582747

Quantum cascade laser dual-comb spectroscopy (DCS) for methane gas mixture studies

Muriel Lepère, Olivier Browet, Sylvain Leonis, Jean Clément, Pitt Allmendinger, Kuno Knapp, Florian Eigenmann, Markus Mangold

Research output: Contribution to conference › Paper

Abstract

For a long time FTIR and laser-based spectroscopies have been used for high resolution molecular spectroscopy studies. The recent development of Dual-Comb Spectroscopy at high resolution (<0.001 cm-1) makes this technique a powerful tool for gas phase studies. The IRis-F1 is a dual-comb spectrometer building on quantum cascade laser frequency combs. We show that it is very well adapted for measurements of line shape parameters. Despite its weak abundance, methane effect on climate and atmospheric chemistry is important. We measured with IRis-F1 the half-widths of absorption lines of methane diluted in nitrogen, and compared with results obtained by other spectroscopies.

Original language	English
DOIs	https://doi.org/10.1117/12.2582747
Publication status	Published - 31 Mar 2021
Event	SPIE BiOS 2021 Digital Forum - Duration: 6 Mar 2021 → 11 Mar 2021 https://www.spie.org/conferences-and-exhibitions/photonics-west/program/conferences/bios?SSO=1

Scientific committee

Scientific committee	SPIE BiOS 2021 Digital Forum
Period	6/03/21 → 11/03/21
Internet address	https://www.spie.org/conferences-and-exhibitions/photonics-west/program/conferences/bios?SSO=1

Keywords

Dual-comb spectroscopy
Gas mixtures
High resolution
Line shape parameters
Methane
Mid-infrared
Quantum cascade laser

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1117/12.2582747

Cite this

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title = "Quantum cascade laser dual-comb spectroscopy (DCS) for methane gas mixture studies",

abstract = "For a long time FTIR and laser-based spectroscopies have been used for high resolution molecular spectroscopy studies. The recent development of Dual-Comb Spectroscopy at high resolution (<0.001 cm-1) makes this technique a powerful tool for gas phase studies. The IRis-F1 is a dual-comb spectrometer building on quantum cascade laser frequency combs. We show that it is very well adapted for measurements of line shape parameters. Despite its weak abundance, methane effect on climate and atmospheric chemistry is important. We measured with IRis-F1 the half-widths of absorption lines of methane diluted in nitrogen, and compared with results obtained by other spectroscopies.",

keywords = "Dual-comb spectroscopy, Gas mixtures, High resolution, Line shape parameters, Methane, Mid-infrared, Quantum cascade laser",

author = "Muriel Lep{\`e}re and Olivier Browet and Sylvain Leonis and Jean Cl{\'e}ment and Pitt Allmendinger and Kuno Knapp and Florian Eigenmann and Markus Mangold",

note = "Funding Information: M. Lep{\`e}re is acknowledging support from “Fonds de la Recherche Scientifique (F.R.S.-FNRS)”. The authors thank Dr Andreas Hugi, co-founder of IRsweep, and Dr Bastien Vispoel, post-doctoral researcher, for their expertise and help. Publisher Copyright: {\textcopyright} 2021 SPIE.; SPIE BiOS 2021 Digital Forum ; Conference date: 06-03-2021 Through 11-03-2021",

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month = mar,

day = "31",

doi = "10.1117/12.2582747",

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T1 - Quantum cascade laser dual-comb spectroscopy (DCS) for methane gas mixture studies

AU - Lepère, Muriel

AU - Browet, Olivier

AU - Leonis, Sylvain

AU - Clément, Jean

AU - Allmendinger, Pitt

AU - Knapp, Kuno

AU - Eigenmann, Florian

AU - Mangold, Markus

N1 - Funding Information: M. Lepère is acknowledging support from “Fonds de la Recherche Scientifique (F.R.S.-FNRS)”. The authors thank Dr Andreas Hugi, co-founder of IRsweep, and Dr Bastien Vispoel, post-doctoral researcher, for their expertise and help. Publisher Copyright: © 2021 SPIE.

PY - 2021/3/31

Y1 - 2021/3/31

N2 - For a long time FTIR and laser-based spectroscopies have been used for high resolution molecular spectroscopy studies. The recent development of Dual-Comb Spectroscopy at high resolution (<0.001 cm-1) makes this technique a powerful tool for gas phase studies. The IRis-F1 is a dual-comb spectrometer building on quantum cascade laser frequency combs. We show that it is very well adapted for measurements of line shape parameters. Despite its weak abundance, methane effect on climate and atmospheric chemistry is important. We measured with IRis-F1 the half-widths of absorption lines of methane diluted in nitrogen, and compared with results obtained by other spectroscopies.

AB - For a long time FTIR and laser-based spectroscopies have been used for high resolution molecular spectroscopy studies. The recent development of Dual-Comb Spectroscopy at high resolution (<0.001 cm-1) makes this technique a powerful tool for gas phase studies. The IRis-F1 is a dual-comb spectrometer building on quantum cascade laser frequency combs. We show that it is very well adapted for measurements of line shape parameters. Despite its weak abundance, methane effect on climate and atmospheric chemistry is important. We measured with IRis-F1 the half-widths of absorption lines of methane diluted in nitrogen, and compared with results obtained by other spectroscopies.

KW - Dual-comb spectroscopy

KW - Gas mixtures

KW - High resolution

KW - Line shape parameters

KW - Methane

KW - Mid-infrared

KW - Quantum cascade laser

UR - http://www.scopus.com/inward/record.url?scp=85103846420&partnerID=8YFLogxK

U2 - 10.1117/12.2582747

DO - 10.1117/12.2582747

M3 - Paper

T2 - SPIE BiOS 2021 Digital Forum

Y2 - 6 March 2021 through 11 March 2021

ER -

Quantum cascade laser dual-comb spectroscopy (DCS) for methane gas mixture studies

Abstract

Scientific committee

Keywords

UN SDGs

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