TY - JOUR
T1 - Hydrodeoxygenation of Levulinic Acid to γ-Valerolactone over Mesoporous Silica-Supported Cu-Ni Composite Catalysts
AU - Popova, Margarita
AU - Trendafilova, Ivalina
AU - Oykova, Manuela
AU - Mitrev, Yavor
AU - Shestakova, Pavleta
AU - Mihályi, Magdolna R.
AU - Szegedi, Ágnes
N1 - Funding Information:
This work was supported by the Bulgarian National Science Fund, Grant KП-06-KOCT/11, 15.12.2021) and EU COST action CA20127. This work was partially supported by the European Regional Development Fund within the Operational Program Science and Education for Smart Growth 2014–2020 under the Project CoE National center of mechatronics and clean technologies BG05M2OP001-1.001-0008-C01. Support of this work in the framework of the bilateral grant agreement between the Bulgarian Academy of Sciences and the Hungarian Academy of Sciences (IC-HU/02/2022–2023) is gratefully acknowledged. Á. Szegedi and M.R. Mihályi are grateful for the support provided by the Ministry of Innovation and Technology of Hungary from the National Research, Development and Innovation Fund, financed under the 2019-2.1.13-TÉT_IN funding scheme (Project No. 2019-2.1.13-TÉT_IN-2020-00043). Research equipment from the Distributed Research Infrastructure INFRAMAT, part of Bulgarian National Roadmap for Research Infrastructures, supported by the Bulgarian Ministry of Education and Science, was used in this investigation. The project No. 2019-2.1.13-TÉT_IN-2020-00043 provided by the Ministry of Innovation and Technology of Hungary from the National Research, Development and Innovation Fund.
Publisher Copyright:
© 2022 by the authors.
PY - 2022/9
Y1 - 2022/9
N2 - Monometallic (Cu, Ni) and bimetallic (Cu-Ni) catalysts supported on KIT-6 based mesoporous silica/zeolite composites were prepared using the wet impregnation method. The catalysts were characterized using X-ray powder diffraction, N2 physisorption, SEM, solid state NMR and H2-TPR methods. Finely dispersed NiO and CuO were detected after the decomposition of impregnating salt on the silica carrier. The formation of small fractions of ionic Ni2+ and/or Cu2+ species, interacting strongly with the silica supports, was found. The catalysts were studied in the gas-phase upgrading of lignocellulosic biomass-derived levulinic acid (LA) to γ-valerolactone (GVL). The bimetallic, CuNi-KIT-6 catalyst showed 100% LA conversion at 250 °C and atmospheric pressure. The high LA conversion and GVL yield can be attributed to the high specific surface area and finely dispersed Cu-Ni species in the catalyst. Furthermore, the catalyst also exhibited high stability after 24 h of reaction time with a GVL yield above 80% without any significant change in metal dispersion.
AB - Monometallic (Cu, Ni) and bimetallic (Cu-Ni) catalysts supported on KIT-6 based mesoporous silica/zeolite composites were prepared using the wet impregnation method. The catalysts were characterized using X-ray powder diffraction, N2 physisorption, SEM, solid state NMR and H2-TPR methods. Finely dispersed NiO and CuO were detected after the decomposition of impregnating salt on the silica carrier. The formation of small fractions of ionic Ni2+ and/or Cu2+ species, interacting strongly with the silica supports, was found. The catalysts were studied in the gas-phase upgrading of lignocellulosic biomass-derived levulinic acid (LA) to γ-valerolactone (GVL). The bimetallic, CuNi-KIT-6 catalyst showed 100% LA conversion at 250 °C and atmospheric pressure. The high LA conversion and GVL yield can be attributed to the high specific surface area and finely dispersed Cu-Ni species in the catalyst. Furthermore, the catalyst also exhibited high stability after 24 h of reaction time with a GVL yield above 80% without any significant change in metal dispersion.
KW - gas-phase hydrogenation
KW - levulinic acid
KW - lignocellulosic biomass
KW - mesoporous silica composites
KW - solid state NMR
KW - γ-valerolactone
UR - http://www.scopus.com/inward/record.url?scp=85137605302&partnerID=8YFLogxK
U2 - 10.3390/molecules27175383
DO - 10.3390/molecules27175383
M3 - Article
C2 - 36080151
AN - SCOPUS:85137605302
SN - 1420-3049
VL - 27
JO - Molecules
JF - Molecules
IS - 17
M1 - 5383
ER -